Research Areas - (46) Physical Chemistry

Full path: Chemistry > Physical Chemistry

Department(s)/lab(s): School of Chemistry / Bio21 Institute | Mulvaney Nanoscience Laboratory @ UMelb
Summary:

Mulvaney directs the ARC Centre of Excellence in Exciton Science and runs Melbourne's nanoscience laboratory. The group's distinctive capability is single-particle and single-emitter optical spectroscopy: photon-antibunching and blinking statistics from individual quantum dots and perovskite nanocrystals, photothermal and dark-field spectroscopy of individual metal nanoparticles, and the electrochemical control of single-nanocrystal charge state. Applications run from LEDs and solar cells to quantum-dot probes for single-particle tracking in cells. Positioned against the established body of NV-ensemble quantum sensing work β€” DEER, nanoscale NMR and T1 relaxometry protocols operating at pT/sqrt(Hz) field sensitivity β€” his single-emitter photon-statistics measurements share the shot-noise-limited photon-counting methodology of NV-ensemble ODMR readout, and the group's nanocrystal probes are direct competitors/complements to nanodiamond in cellular sensing. Large, well-resourced group.

Department(s)/lab(s): Physics & Astronomy – AMOPP | Quantum Biomolecular Processes Group (Olaya-Castro Group) @ UCL
Summary:

Olaya-Castro leads theoretical research on quantum phenomena in biological systems. Research directions: (1) Quantum coherence in photosynthesis β€” open quantum systems theory for energy transfer in light-harvesting complexes, probing whether quantum coherence provides functional advantage; vibronic coupling models for chromophore-protein complexes; (2) Counting statistics and noise in exciton and charge transfer; (3) Quantum thermodynamics of biomolecular machines β€” efficiency limits and entropy production in molecular motors; (4) Non-classical features of electronic/vibrational dynamics in chromophores; (5) Connections between quantum information measures and biological function. Collaborates with Bain and Llorente-Garcia on joint experiment/theory biosensing projects. Theoretical work only β€” no experimental activity.

Department(s)/lab(s): Physics | LuMIn - Nanoplasmonics & Ultrafast (Palpant) @ ENSPS
Summary:

Palpant (current LuMIn director) studies ultrafast optical response and thermoplasmonics of metal nanoparticles - photothermal nanoscale heat sources and sensors for photonics and biomedicine. Primary appointment CentraleSupelec; based at the ENS Paris-Saclay LuMIn site. In the broader landscape of NV-centre ensemble quantum sensing (DEER, nano-NMR, T1 relaxometry) operating near pT/sqrt(Hz) sensitivity, this work is adjacent through plasmonic photothermal transduction and sensing.

Department(s)/lab(s): Physics & Astronomy – Photon Science Institute | Parkinson Group (Ultrafast Spectroscopy of Photonic Materials) @ Manchester
Summary:

Parkinson's group uses ultrafast optical spectroscopy to study carrier dynamics in photonic materials with quantum device applications. Research directions: (1) Time-resolved photoluminescence β€” TRPL with single-photon counting to map exciton lifetimes, diffusion, and defect trapping in GaN, perovskite, and 2D semiconductor quantum wells; (2) Optical single-particle spectroscopy β€” isolating single nanowires or nanocrystals for defect-free measurements of intrinsic optical properties; (3) Photon-number statistics β€” Hanbury Brown–Twiss measurements of single-photon purity from quantum dots and localized excitons; (4) Semiconductor quantum sensing interfaces β€” studying how carrier dynamics affect the fidelity of semiconductor-based quantum sensors and emitters.

Department(s)/lab(s): Physics (Cavendish Laboratory) | Rao Group - Optoelectronics @ Cambridge
Summary:

Rao's group uses ultrafast (sub-20 fs) transient absorption and vibronic spectroscopy to study quantum-coherent energy and charge transfer processes in molecular and nanoscale semiconductor systems, most notably the quantum-coherent mechanism of singlet exciton fission, with applications to next-generation photovoltaics.

Department(s)/lab(s): Physics | Photonics and Complex Media Group (Sapienza) @ Imperial
Summary:

Sapienza studies light propagation and control in complex/disordered nanophotonic media, using wavefront shaping and transmission-matrix approaches to focus and image through scattering media, with applications to deep-tissue fluorescence imaging and nanophotonic light sources.

Department(s)/lab(s): Chemistry | Scholes Group @ Princeton
Summary:

Scholes uses multidimensional ultrafast and coherence spectroscopies to probe wavepacket dynamics and quantum-mechanical phenomena in photosynthetic light-harvesting complexes, cavity QED, and photo-activated chemistry, including his group's resolution of a decade-long controversy over long-lived coherent coupling in the Fenna-Matthews-Olson complex. His current work extends coherence spectroscopy to quantum information science and photobiomodulation, squarely fitting the fundamental light-physics/quantum-optics side of the filter.

Department(s)/lab(s): School of Chemistry | Smith Time-Resolved Spectroscopy and Microspectroscopy Group @ UMelb
Summary:

Smith runs Melbourne's time-resolved fluorescence facility and specialises in the information channels most people throw away: fluorescence lifetime, anisotropy decay and its orientational content, and single-molecule photophysics, applied to organic semiconductors, energy-transfer systems and biological samples. The group builds its own confocal microspectroscopy instrumentation for time-resolved anisotropy imaging and single-molecule detection. Positioned against the established body of NV-ensemble quantum sensing work β€” DEER, nanoscale NMR and T1 relaxometry protocols operating at pT/sqrt(Hz) field sensitivity β€” lifetime- and orientation-resolved fluorescence is the principal orthogonal contrast mechanism to spin-based sensing, and his instrumentation is the natural correlative partner for NV-ensemble DEER/relaxometry experiments at pT/sqrt(Hz) that need an independent optical readout of the same specimen. Preferred attribute present: orientation- and lifetime-resolved methods.

Department(s)/lab(s): Physics & Astronomy | Sokolov Laboratory (IQSE) @ TAMU
Summary:

Sokolov develops femtosecond adaptive spectroscopic techniques for coherent Raman (FAST CARS), broadband stochastic laser fields, and quantum-light probes of molecular coherence for standoff chemical/biological sensing and label-free imaging. In the broader landscape of NV-centre ensemble quantum sensing (DEER, nano-NMR, T1 relaxometry) operating near pT/sqrt(Hz) sensitivity, this work contributes ultrafast coherent-Raman methodology adjacent to spin-based sensing.

Department(s)/lab(s): Chemistry | Tempelaar Team @ Northwestern
Summary:

Tempelaar develops theory and simulation methods (surface-hopping and vibronic exciton models) for two-dimensional electronic spectroscopy, explaining how vibronic coupling sustains excitonic coherence in photosynthetic light-harvesting complexes such as the Fenna-Matthews-Olson complex and LH2, and extending these ideas to singlet fission and organic-semiconductor aggregates. He is a faculty affiliate of Northwestern's Institute for Quantum Information Research and Engineering (INQUIRE).