Description: Ultrashort pulse spectroscopies (transient absorption, 2D-ES, attosecond transient absorption) to probe electron and nuclear dynamics on fsβas timescales.
Boland's group focuses on THz spectroscopy of semiconductor nanostructures and 2D materials for quantum sensing applications. Research directions: (1) THz optical pumpβTHz probe spectroscopy β measuring ultrafast carrier dynamics in semiconductor nanowires, quantum wells, and 2D materials (graphene, TMDs, perovskites) after optical excitation; (2) Near-field THz nanoscopy β sub-wavelength THz imaging of carrier distributions and quantum phase domains; (3) THz-active quantum devices β studying exciton and polaron dynamics in perovskite and III-V semiconductors at THz frequencies; (4) 2D material sensors β graphene-based THz detectors and emitters. Applications in quantum-material characterization and quantum sensing.
Prof. Gaynor (Chemistry, joined summer 2023) develops cutting-edge ultrafast spectroscopy at the physics-chemistry frontier. Directions: (1) Attochemistry β new ultrafast laser spectroscopies operating on attosecond to femtosecond timescales to directly measure how electron spin and orbital motion couple to molecular geometry (spin-vibronic coupling) in chiral molecules and materials of interest for energy conversion and spintronics; (2) Multidimensional nonlinear spectroscopy (2D electronic spectroscopy, 2D vibrational) to track energy and charge transfer immediately after photoexcitation; (3) Instrumentation-first approach: building novel attosecond transient absorption and correlation spectroscopy apparatus from scratch, enabling entirely new observables (e.g., electron-nuclear and spin-orbital correlations). INQUIRE faculty affiliate. Beckman Young Investigator 2025 ($600k, 4 yrs); Packard Fellow 2025 ($875k, 5 yrs).
Halsall is a senior PSI photonics researcher focusing on semiconductor spectroscopy and photonic quantum device characterization. Research directions: (1) Deep-level transient spectroscopy (DLTS) β characterizing defects and impurities in semiconductor quantum device structures (Si, GaN, SiC) that are relevant to qubit coherence; (2) Photoluminescence mapping β spatial mapping of optical quality in quantum well and dot wafers for quantum sensing device development; (3) InGaN/GaN quantum wells β non-destructive optical characterization of LED and sensor structures; (4) THz and infrared spectroscopy β contactless Hall measurements and Drude response for quantum material characterization. Provides photonic metrology tools for characterizing quantum sensing device materials.
Hibberd holds an EPSRC Ernest Rutherford Fellowship at Manchester's PSI. Research directions: (1) Ultrafast THz spectroscopy of magnetic materials β probing spin dynamics, magnon modes, and phase transitions in correlated magnetic materials with sub-ps time resolution using intense THz pulses; (2) THz-driven spintronics β using THz electric and magnetic fields to switch magnetization and induce spin currents; (3) THz generation from spintronic heterostructures β using ultrafast spin-charge conversion as a broadband THz emitter for materials characterization; (4) Quantum magnonics β studying collective spin excitations (magnons) as quantum sensors of materials order parameters. Bridges ultrafast optics and quantum sensing of magnetic phases.
Leone's group generates attosecond and few-femtosecond XUV/X-ray pulses to track electron dynamics and charge migration in molecules and materials in real time, pushing time-domain spectroscopy toward the natural timescale of electronic motion.
Parkinson's group uses ultrafast optical spectroscopy to study carrier dynamics in photonic materials with quantum device applications. Research directions: (1) Time-resolved photoluminescence β TRPL with single-photon counting to map exciton lifetimes, diffusion, and defect trapping in GaN, perovskite, and 2D semiconductor quantum wells; (2) Optical single-particle spectroscopy β isolating single nanowires or nanocrystals for defect-free measurements of intrinsic optical properties; (3) Photon-number statistics β Hanbury BrownβTwiss measurements of single-photon purity from quantum dots and localized excitons; (4) Semiconductor quantum sensing interfaces β studying how carrier dynamics affect the fidelity of semiconductor-based quantum sensors and emitters.
Scholes uses multidimensional ultrafast and coherence spectroscopies to probe wavepacket dynamics and quantum-mechanical phenomena in photosynthetic light-harvesting complexes, cavity QED, and photo-activated chemistry, including his group's resolution of a decade-long controversy over long-lived coherent coupling in the Fenna-Matthews-Olson complex. His current work extends coherence spectroscopy to quantum information science and photobiomodulation, squarely fitting the fundamental light-physics/quantum-optics side of the filter.