Description: Multi-frequency pulsed electron paramagnetic resonance including dynamical decoupling, ENDOR, and DEER/PELDOR for measuring coherence and inter-qubit couplings in molecular spin systems.
van Slageren's group is one of the leading molecular-qubit labs. They synthesize their own paramagnetic molecules, characterize them with a wide spectroscopic and magnetometric arsenal (multi-frequency and high-field EPR, pulsed EPR/DEER, THz spectroscopy, SQUID magnetometry) and back it with ab-initio calculation. Landmarks include room-temperature quantum coherence in a copper(II) molecular qubit, quantitative prediction of nuclear-spin-diffusion-limited coherence times, measurement of coherence in thin films without post-processing, and recent observation of a sizeable spin-electric effect -- electric-field control of a molecular spin state, which is the mechanism you would exploit for a molecular electrometer. Current direction: molecular quantum spintronics, marrying organic spintronics to molecular magnetism. Relative to the established NV-ensemble quantum-sensing playbook (DEER, nanoscale NMR, T1 relaxometry at pT/sqrt(Hz) ensemble sensitivity), this is the molecular alternative to the diamond defect: chemically tunable spin qubits whose coherence can be engineered by ligand design rather than by host-crystal purification. Immediate neighbours are Krueger (nanodiamond chemistry) and Wrachtrup (NV readout), both already on file -- an unusually complete local ecosystem.
Winpenny holds the Regius Chair in Chemistry at Manchester and is a world leader in molecular magnetism and molecular nanomagnets for quantum technologies. Research directions: (1) Molecular nanomagnets — synthesis of Cr7Ni 'horseshoe' rings and related cage clusters as prototype molecular qubits with long T2 times; (2) Multi-qubit molecular architectures — covalently linked molecular qubit pairs and arrays for quantum gate operations and distributed sensing; (3) Quantum error correction in molecules — designing molecular systems encoding logical qubits with error protection; (4) Quantum sensing applications — molecular spin systems as ultra-sensitive nanoscale magnetic sensors in the sub-nm regime. Leading the NPL M4Q Network and UK molecular qubit community.