Loth combines ESR-STM with ultrafast terahertz-driven STM to read out and control individual atomic and molecular spins with atomic spatial and picosecond temporal resolution - single-spin quantum sensing at the ultimate spatial limit. In the broader landscape of NV-centre ensemble quantum sensing (DEER, nano-NMR, T1 relaxometry) operating near pT/sqrt(Hz) sensitivity, this work pushes spin sensing to the single-atom, ultrafast regime.